From rungs to ribbons
Pile lots of atoms into a crystal and the discrete energy rungs of each atom merge into wide bands. The highest filled band is called the valence band; the next-empty one above it is the conduction band; the gap between them — the band gap Eg — is what makes the crystal a semiconductor.
Below the gap, the crystal is transparent: there is no available electronic state for the photon to drop into. Above the gap, an electron is kicked from the valence band into the conduction band, leaving behind a hole.
Why we care
Three direct consequences for this experiment:
- CrSBr's band gap (~1.5 eV) sets the energy below which the material itself is roughly transparent.
- Just below the gap an exciton appears — a bound state that gives the sharpest absorption feature in the system.
- The whole optical fingerprint of CrSBr (its dielectric function) is dominated by physics happening near this gap.
Key takeaways
- Crystals quantise allowed energies into bands.
- The band gap controls absorption onset and exciton position.